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Functionalization of 3D printed ABS filters with MOF for toxic gas removal

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dc.contributor.authorPellejero, Ismael
dc.contributor.authorAlmazán, Fernandoes_ES
dc.contributor.authorLafuente, Maríaes_ES
dc.contributor.authorUrbiztondo, Miguel A.es_ES
dc.contributor.authorDobrek, Martines_ES
dc.contributor.authorBechelany, Mikhaeles_ES
dc.contributor.authorJulbe, Annees_ES
dc.contributor.authorGandía Pascual, Luis
dc.contributor.departmentInstitute for Advanced Materials and Mathematics - INAMAT2en
dc.contributor.funderGobierno de Navarra / Nafarroako Gobernua, PC052-23es
dc.contributor.funderUniversidad Pública de Navarra / Nafarroako Unibertsitate Publikoaes
dc.date.accessioned2020-11-27T08:45:56Z
dc.date.available2022-09-25T23:00:12Z
dc.date.issued2020
dc.description.abstractAcrylonitrile butadiene styrene (ABS) is one of the most extensively used polymer in 3D printing manufacturing due to its competitive thermal and mechanical properties. Recently, a special attention has been devoted to novel ABS composites featuring extra functionalities e.g. in the area of VOC removal. Herein, we report on a facile protocol for the functionalization of 3D printed ABS filters with a MOF (Metal- Organic Framework) material (ZIF-8) targeting the conception of attractive gas filters. The proposed synthesis strategy consists in low temperature ALD (Atomic Layer Deposition) of ZnO on the ABS grid followed by the hydrothermal conversion of ZnO to ZIF-8, both steps being conducted at 60 °C. In such way, the method enables an effective growth of ZIF-8 without altering the stability of the polymeric ABS support. The as-fabricated ABS/ZIF-8 filters offer a promising adsorption behaviour for dimethyl methylphosphonate (~20.4 mg of DMMP per gram of ZIF-8), thus proving their potential for toxic gas capture applications.en
dc.description.sponsorshipFinancial support from Gobierno de Navarra (grants PC052-23), from MINECO (grant CTQ2016-79419-R) and from the Spanish Ministerio de Ciencia, Innovación y Universidades and the European Regional Development Fund (ERDF/FEDER) (grant RTI2018-096294-B-C31) is gratefully acknowledged. I.P. thanks Obra Social la Caixa, Fundación Caja Navarra and UPNA for his research contracts in the framework of the programs 'Ayudas Postdoctorales' and 'CaptaciónTalento'. L. M. G. wishes to thank Banco de Santander and Universidad Pública de Navarra for their financial support under 'Programa de Intensificación de la Investigación 2018' initiative.en
dc.embargo.lift2022-09-25
dc.embargo.terms2022-09-25
dc.format.extent31 p.
dc.format.mimetypeapplication/pdfen
dc.identifier.doi10.1016/j.jiec.2020.05.013
dc.identifier.issn1226-086X
dc.identifier.urihttps://academica-e.unavarra.es/handle/2454/38796
dc.language.isoengen
dc.publisherElsevieren
dc.relation.ispartofJournal of Industrial and Engineering Chemistry 89 (2020) 194-203en
dc.relation.projectIDinfo:eu-repo/grantAgreement/ES/1PE/CTQ2016-79419-Ren
dc.relation.publisherversionhttps://doi.org/10.1016/j.jiec.2020.05.013
dc.rights© 2020 The Korean Society of Industrial and Engineering Chemistry. Published by Elsevier B.V. This manuscript version is made available under the CC-BY-NC-ND 4.0en
dc.rights.accessRightsinfo:eu-repo/semantics/openAccessen
dc.rights.accessRightsAcceso abierto / Sarbide irekiaes
dc.subjectZIF-8en
dc.subject3D printingen
dc.subjectABS filteren
dc.subjectAtomic layer depositionen
dc.subjectVOCs abatementen
dc.subjectGas treatmenten
dc.titleFunctionalization of 3D printed ABS filters with MOF for toxic gas removalen
dc.typeinfo:eu-repo/semantics/articleen
dc.typeArtículo / Artikuluaes
dc.type.versioninfo:eu-repo/semantics/acceptedVersionen
dc.type.versionVersión aceptada / Onetsi den bertsioaes
dspace.entity.typePublication
relation.isAuthorOfPublicationb4cb3430-7b46-428d-8714-7d9af415aebf
relation.isAuthorOfPublicationd2bd5a4b-ea1f-488b-afea-05b77f69d3f0
relation.isAuthorOfPublication.latestForDiscoveryb4cb3430-7b46-428d-8714-7d9af415aebf

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