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Magnetically activated 3D printable polylactic acid/polycaprolactone/magnetite composites for magnetic induction heating generation

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dc.contributor.authorGalarreta Rodríguez, Itziar
dc.contributor.authorLópez Ortega, Alberto
dc.contributor.authorGarayo Urabayen, Eneko
dc.contributor.authorBeato López, Juan Jesús
dc.contributor.authorLa Roca, Paulo Matías
dc.contributor.authorSánchez-Alarcos Gómez, Vicente
dc.contributor.authorRecarte Callado, Vicente
dc.contributor.authorGómez Polo, Cristina
dc.contributor.authorPérez de Landazábal Berganzo, José Ignacio
dc.contributor.departmentCienciases_ES
dc.contributor.departmentZientziakeu
dc.contributor.departmentInstitute for Advanced Materials and Mathematics - INAMAT2en
dc.contributor.funderUniversidad Pública de Navarra / Nafarroako Unibertsitate Publikoaes
dc.date.accessioned2023-06-15T12:12:12Z
dc.date.available2023-06-15T12:12:12Z
dc.date.issued2023
dc.date.updated2023-06-15T11:36:39Z
dc.description.abstractAdditive manufacturing technology has attracted the attention of industrial and technological sectors due to the versatility of the design and the easy manufacture of structural and functional elements based on composite materials. The embedding of magnetic nanoparticles in the polymeric matrix enables the development of an easy manufacturing process of low-cost magnetically active novel polymeric composites. In this work, we report a series of magnetic composites prepared by solution casting method combining 5 to 60 wt.% of 140 ± 50 nm commercial Fe3O4 nanoparticles, with a semi-crystalline, biocompatible, and biodegradable polymeric blend made of polylactic acid (PLA) and polycaprolactone (PCL). The composites were extruded, obtaining 1.5 ± 0.2 mm diameter continuous and flexible filaments for fused deposition modelling 3D printing. The chemical, magnetic, and calorimetric properties of the obtained filaments were investigated by differential scanning calorimetry, thermogravimetric analysis, magnetometry, and scanning electron microscopy. Furthermore, taking advantage of the magnetic character of the filaments, their capability to generate heat under the application of low-frequency alternating magnetic fields (magnetic induction heating) was analyzed. The obtained results expose the versatility of these easy manufacturing and low-cost filaments, where selecting a desired composition, the heating capacity can be properly adjusted for those applications where magnetic induction plays a key role (i.e., magnetic hyperthermia, drug release, heterogeneous catalysis, water electrolysis, gas capture, or materials synthesis).en
dc.description.sponsorshipOpen Access funding provided by Universidad Pública de Navarra. This work has been carried out with the financial support of the Navarra Government (project number PC017-018 AMELEC). The Spanish Government is acknowledged for the HIPERNANO research network (RED2018-102626-T). ALO acknowledges financial support from the grants PID2021-122613OB-I00 funded by MCIN/AEI/10.13039/501100011033 and PJUPNA2020 from Universidad Pública de Navarra. P. La Roca has received funding from “la Caixa” and “Caja Navarra” Foundations, under agreement LCF/PR/PR13/51080004.en
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dc.identifier.citationGalarreta-Rodriguez, I., Lopez-Ortega, A., Garayo, E., Beato-López, J. J., La Roca, P., Sanchez-Alarcos, V., Recarte, V., Gómez-Polo, C., & Pérez-Landazábal, J. I. (2023). Magnetically activated 3D printable polylactic acid/polycaprolactone/magnetite composites for magnetic induction heating generation. Advanced Composites and Hybrid Materials, 6(3), 102. https://doi.org/10.1007/s42114-023-00687-4en
dc.identifier.doi10.1007/s42114-023-00687-4
dc.identifier.issn2522-0128
dc.identifier.urihttps://academica-e.unavarra.es/handle/2454/45488
dc.language.isoengen
dc.publisherSpringeren
dc.relation.ispartofAdvanced Composites and Hybrid Materials (2023) 6:102en
dc.relation.projectIDinfo:eu-repo/grantAgreement/AEI/Plan Estatal de Investigación Científica y Técnica y de Innovación 2013-2016/RED2018-102626-Ten
dc.relation.projectIDinfo:eu-repo/grantAgreement/AEI/Plan Estatal de Investigación Científica y Técnica y de Innovación 2021-2023/PID2021-122613OB-I00en
dc.relation.projectIDinfo:eu-repo/grantAgreement/Gobierno de Navarra//PC017-018en
dc.relation.publisherversionhttps://doi.org/10.1007/s42114-023-00687-4
dc.rights© The Author(s) 2023. This article is licensed under a Creative Commons Attribution 4.0 International License, which permits use, sharing, adaptation, distribution and reproduction in any medium or format, as long as you give appropriate credit to the original author(s) and the source, provide a link to the Creative Commons licence, and indicate if changes were made. The images or other third party material in this article are included in the article's Creative Commons licence, unless indicated otherwise in a credit line to the material. If material is not included in the article's Creative Commons licence and your intended use is not permitted by statutory regulation or exceeds the permitted use, you will need to obtain permission directlyen
dc.rights.accessRightsAcceso abierto / Sarbide irekiaes
dc.rights.accessRightsinfo:eu-repo/semantics/openAccessen
dc.rights.urihttp://creativecommons.org/licenses/by/4.0/
dc.subjectMagnetic nanoparticlesen
dc.subjectComposite materialsen
dc.subjectMagnetic filamentsen
dc.subjectFused deposition modellingen
dc.subject3D printingen
dc.titleMagnetically activated 3D printable polylactic acid/polycaprolactone/magnetite composites for magnetic induction heating generationen
dc.typeArtículo / Artikuluaes
dc.typeinfo:eu-repo/semantics/articleen
dc.type.versionVersión publicada / Argitaratu den bertsioaes
dc.type.versioninfo:eu-repo/semantics/publishedVersionen
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